I checked the back of my Samsung charger yesterday and it was actually 5.3v @ 2a. I tried a 5.0v charger with the VS data cable and now it stays at 1.96-1.99a without hitting 0.
However, I also changed the charging screen to show USB voltage and it was at 4.58v instead of 4.2 like the charge-only cables. With the 5.3v charger and data cable it was at 4.83-5.2v but constantly fluctuating amps to regulate the current.
Data cable
5v charger:
4.58v
1.82-1.99A (usually 1.96-1.99)
8.5-9w
5.3v charger:
4.83v (hits 5v briefly every 30-90sec)
1.5-1.95A (drops to 0a @ 5v)
8.0-9.5w/(0-4w @ 5v)
Charge-only cable
5v charger:
4.26v
1.3-1.4a
5.5-6w
5.3v charger:
4.31v
1.92-1.99a
8.5w
So it appears the charger shuts off above 5v, but the VS data cable allows it to reach those voltages with a 5v+ charger. The charge-only cables stay around 4.2v (I tested 2 with the exact same numbers), but only hits 1.3-1.4a with the 5.0v charger vs 1.99a with the 5.3v charger.
I think the reason for this is the short VS data cable is 20AWG rated at 2.4a while my old charge-only cables are probably 24-28AWG and only capable of 1.3-1.6a @ 5v due to more internal resistance, voltage drop and length. The 5.3v Samsung charger is compensating for that voltage drop by overloading the cable (pushing more current at lower voltage), causing it to stop charging early since the supply voltage must be greater than the battery voltage (see this link where he specifically mentions the 94% I was seeing
USB Cable Resistance: Why your phone/tablet might be charging slow)
TL;DR - Use a 20AWG cable and 5.0v charger for best performance. A 5.3v charger will appear to be working, but actually charges slower with a 20AWG cable due to fluctuating current and may push 24-28AWG cables too hard causing it to stop charging early.